This model demonstrates the attosecond transient absorption spectra computed using the following formula: $$ \sigma (\omega,\tau) = \frac{4\pi\omega}{c} \text{Im} \sum_I \sum_J c_I c_J \exp\left( i (E_I - E_J) \tau \right) \sum_F \langle \Phi_I | \hat{\mu} | \Phi_F \rangle \langle \Phi_F | \hat{\mu} | \Phi_J \rangle \left( \frac{1}{\tilde{E}_F - E_I - \omega} + \frac{1}{\tilde{E}^*_F - E_J + \omega} \right) $$ See the references listed below for a detailed discussion:
  1. R. Santra et al., Phys. Rev. A 83, 033405 (2011)
  2. N. Golubev et al., Phys. Rev. Lett. 127, 123001 (2021)
System Energy Levels
Transition Dipole Moments & Population

$$\langle \Phi_1 | \hat{\mu} | \Phi_{F_1} \rangle =$$

$$\langle \Phi_1 | \hat{\mu} | \Phi_{F_2} \rangle =$$

$$\langle \Phi_2 | \hat{\mu} | \Phi_{F_1} \rangle =$$

$$\langle \Phi_2 | \hat{\mu} | \Phi_{F_2} \rangle =$$

$$c^2_1 =$$

Attosecond Transient Absorption Spectrum
Energy-Resolved Lineouts

Welcome to the Attosecond Transient Absorption Spectroscopy (ATAS) Learning Tool!

Developers: Nikolay Golubev

This interactive tool demonstrates how attosecond transient absorption spectroscopy (ATAS) can be used to probe coherent electron dynamics in a quantum system prepared in a superposition of its two lowest-energy states. The two higher-lying states act as final states for the absorption process, giving rise to distinct spectral features. By adjusting the system parameters, explore how the populations, coherences, and relative phases of the quantum states influence the amplitudes and phases of the corresponding absorption transitions.

For additional interactive demonstrations and related projects, visit www.ngolubev.com!